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Techno-economic evaluation of a biogas-based oxidative coupling of methane process for ethylene production

Alberto T. Penteado, Mijin Kim, Hamid R. Godini, Erik Esche, Jens-Uwe Repke

《化学科学与工程前沿（英文）》 2018年 第12卷 第4期   页码 598-618 doi: 10.1007/s11705-018-1752-5

摘要：

This contribution is a preliminary techno-economic assessment of a biogas-based oxidative coupling of methane (OCM) process. Biogas is frequently utilized as a renewable energy source within small scale combined heat and power plants or as a natural gas substitute. The activation of methane also enables its utilization as a feedstock to produce chemicals. In this sense, the OCM process allows for the direct conversion of methane into ethylene, which is a major building block for the chemical and polymer industries. Biogas resulting from the anaerobic digestion of vinasse, a liquid effluent from bioethanol industry, is treated for contaminant removal and its methane content is converted into ethylene, which is then purified as the main product. The biogas cleaning process is assessed based on literature data, while an experimentally validated simulation model is used to assess the OCM process. A techno-economic evaluation is then performed through a Monte Carlo simulation, wherein uncertain parameters take random values between reasonable bounds. The net present value results positive in 74% of the cases, indicating that the project is profitable under a wide range of scenarios. Some performance improvement opportunities have been identified and highlighted to guide future studies in the topic.

关键词： biogas conversion     ethylene production     oxidative coupling of methane     feasibility study    

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Dehydration of natural gas and biogas streams using solid desiccants: a review

Soheil Bahraminia, Mansoor Anbia, Esmat Koohsaryan

《化学科学与工程前沿（英文）》 2021年 第15卷 第5期   页码 1050-1074 doi: 10.1007/s11705-020-2025-7

摘要： Natural gas and biogas are two mixtures that consist of methane as their main component. These two gas mixtures are usually saturated with water vapor, which cause many problems, such as damaging the gas processing equipment by increasing the gas’s corrosion potential or clogging the pipelines due to gas hydrate formation. Thus, removing water vapor from these gas streams is mandatory. In this review paper, the main dehydration methods have been overviewed, and scrutiny of the adsorption dehydration has been carried out. Furthermore, the most important solid desiccants and their improvements have been reviewed.

关键词： natural gas     biogas     dehydration     adsorption     solid desiccant    

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Distribution of PCDD/Fs in a food waste anaerobic digestion process with biogas utilization

《环境科学与工程前沿（英文）》 2023年 第17卷 第11期 doi: 10.1007/s11783-023-1736-7

摘要：

● The PCDD/F distribution patterns of the FW-AD process were investigated.

关键词： Biological treatment     MSW classification     Mass balance     Solid digestate    

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大型养殖场沼气工程

潘文智

《中国工程科学》 2011年 第13卷 第2期   页码 40-43

摘要：

结合国内外大中型沼气工程情况，以德青源沼气工程为例，介绍了农村废弃物变废为宝的工艺流程，提供了农村能源解决方案，并结合我国沼气工程现有问题提出几点建议，以使大中型沼气工程走向规范化。

关键词： 沼气工程     德青源沼气工程     核心技术     展望与建议    

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Influence of HS and NH on biogas dry reforming using Ni catalyst: a study on single and synergetic effect

《环境科学与工程前沿（英文）》 2023年 第17卷 第3期 doi: 10.1007/s11783-023-1632-1

摘要：

● NH3 in biogas had a slight inhibitory effect on dry reforming.

关键词： Biogas     Dry reforming     Sulfur poisoning     Ammonia     Synergetic effect     Hydrogen    

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VALORIZATION OF BIOGAS THROUGH SIMULTANEOUS CO AND HS REMOVAL BY RENEWABLE AQUEOUS AMMONIA SOLUTION IN

《农业科学与工程前沿（英文）》 2023年 第10卷 第3期   页码 468-478 doi: 10.15302/J-FASE-2022473

摘要：

● Simultaneous H2S and CO2 removal from biogas is studied.

关键词： biomethane     biogas purification     CO2 removal     H2S removal     membrane absorption    

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Techno-economic assessment of providing control energy reserves with a biogas plant

Ervin Saracevic, David Woess, Franz Theuretzbacher, Anton Friedl, Angela Miltner

《化学科学与工程前沿（英文）》 2018年 第12卷 第4期   页码 763-771 doi: 10.1007/s11705-018-1776-x

摘要：

Grid stability is being challenged by the increasing integration of power plants with volatile power generation into the energy system. Power supply fluctuations must be compensated by energy system flexibility. The storability of the energy carrier enables biogas plants to generate power flexibly. In this study, the technical and economic effects of providing positive secondary control energy reserves with an Austrian biogas plant were assessed. The plant’s main focus lies in biomethane production with the option of heat and power generation through combined heat and power (CHP) units. A detailed simulation model of the investigated biogas plant was developed, which is presented in this work. Ex-post simulations of one year of flexible plant operation were conducted with this model. The findings show that the installed biogas storage capacity is sufficient to provide control energy reserves while simultaneously producing biomethane. Profitability of providing control energy reserves largely depends on the prices at the control energy market and on CHP unit start-up costs. A cost efficiency analysis demonstrated that investing in a hot water tank with a volume of 5 m3 for short-term heat storage turned out to be economically viable.

关键词： biogas plant     process simulation     control energy reserves     economic assessment     gas storage    

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Biogas and its opportunities—A review

Panagiotis G. Kougias, Irini Angelidaki

《环境科学与工程前沿（英文）》 2018年 第12卷 第3期 doi: 10.1007/s11783-018-1037-8

摘要： Biogas production is a well-established technology primarily for the generation of renewable energy and also for the valorization of organic residues. Biogas is the end product of a biological mediated process, the so called anaerobic digestion, in which different microorganisms, follow diverse metabolic pathways to decompose the organic matter. The process has been known since ancient times and was widely applied at domestic households providing heat and power for hundreds of years. Nowadays, the biogas sector is rapidly growing and novel achievements create the foundation for constituting biogas plants as advanced bioenergy factories. In this context, the biogas plants are the basis of a circular economy concept targeting nutrients recycling, reduction of greenhouse gas emissions and biorefinery purposes. This review summarizes the current state-of-the-art and presents future perspectives related to the anaerobic digestion process for biogas production. Moreover, a historical retrospective of biogas sector from the early years of its development till its recent advancements gives an outlook of the opportunities that are opening up for process optimisation.

关键词： Anaerobic digestion     Biogas     Biowastes     Solid waste     Manure     Industrial waste    

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Hydrogel photocatalysts for efficient energy conversion and environmental treatment

《能源前沿（英文）》 2021年 第15卷 第3期   页码 577-595 doi: 10.1007/s11708-021-0756-x

摘要： Photocatalysts have attracted great research interest owing to their excellent properties and potential for simultaneously addressing challenges related to energy needs and environmental pollution. Photocatalytic particles need to be in contact with their respective media to exhibit efficient photocatalytic performances. However, it is difficult to separate nanometer-sized photocatalytic materials from reaction media later, which may lead to secondary pollution and a poor recycling performance. Hydrogel photocatalysts with a three-dimensional (3D) network structures are promising support materials for photocatalysts based on features such as high specific surface areas and adsorption capacities and good environmental compatibility. In this review, hydrogel photocatalysts are classified into two different categories depending on their elemental composition and recent progresses in the methods for preparing hydrogel photocatalysts are summarized. Moreover, current applications of hydrogel photocatalysts in energy conversion and environmental remediation are reviewed. Furthermore, a comprehensive outlook and highlight future challenges in the development of hydrogel photocatalysts are presented.

关键词： hydrogel     photocatalysts     energy conversion     environmental treatment    

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Biological conversion pathways of sulfate reduction ammonium oxidation in anammox consortia

Zhen Bi, Deqing Wanyan, Xiang Li, Yong Huang

《环境科学与工程前沿（英文）》 2020年 第14卷 第3期 doi: 10.1007/s11783-019-1217-1

摘要： The SRAO phenomena tended to occur only under certain conditions. High amount of biomass and non-anaerobic condition is requirement for SRAO. Anammox bacteria cannot oxidize ammonium with sulfate as electron acceptor. AOB and AnAOB are mainly responsible for ammonium conversion. Heterotrophic sulfate reduction mainly contributed to sulfate conversion. For over two decades, sulfate reduction with ammonium oxidation (SRAO) had been reported from laboratory experiments. SRAO was considered an autotrophic process mediated by anammox bacteria, in which ammonium as electron donor was oxidized by the electron acceptor sulfate. This process had been attributed to observed transformations of nitrogenous and sulfurous compounds in natural environments. Results obtained differed largely for the conversion mole ratios (ammonium/sulfate), and even the intermediate and final products of sulfate reduction. Thus, the hypothesis of biological conversion pathways of ammonium and sulfate in anammox consortia is implausible. In this study, continuous reactor experiments (with working volume of 3.8L) and batch tests were conducted under normal anaerobic (0.2≤DO<0.5 mg/L) / strict anaerobic (DO<0.2 mg/L) conditions with different biomass proportions to verify the SRAO phenomena and identify possible pathways behind substrate conversion. Key findings were that SRAO occurred only in cases of high amounts of inoculant biomass under normal anaerobic condition, while absent under strict anaerobic conditions for same anammox consortia. Mass balance and stoichiometry were checked based on experimental results and the thermodynamics proposed by previous studies were critically discussed. Thus anammox bacteria do not possess the ability to oxidize ammonium with sulfate as electron acceptor and the assumed SRAO could, in fact, be a combination of aerobic ammonium oxidation, anammox and heterotrophic sulfate reduction processes.

关键词： Anammox bacteria     Autotrophic     Biological conversion     Sulfate reducing ammonium oxidation (SRAO)    

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Sustainable conversion regenerated cellulose into cellulose oleate by sonochemistry

《化学科学与工程前沿（英文）》 2023年 第17卷 第8期   页码 1096-1108 doi: 10.1007/s11705-023-2317-9

摘要： Derivatization has great potential for the high-value utilization of cellulose by enhancing its processability and functionality. However, due to the low reactivity of natural cellulose, it remains challenging to rapidly prepare cellulose derivatives with high degrees of substitution. The “cavitation effect” of ultrasound can reduce the particle size and crystalline index of cellulose, which provides a possible method for preparing cellulose derivatives. Herein, a feasible method was proposed for efficiently converting regenerated cellulose to cellulose oleate with the assistance of ultrasonic treatment. By adjusting the reaction conditions including ultrasonic intensity, feeding ratios of oleic acid, reaction time, and reaction solvent, a series of cellulose oleates with degrees of substitution ranging from 0.37 to 1.71 were synthesized. Additionally, the effects of different reaction conditions on the chemical structures, crystalline structures, and thermal behaviors were investigated thoroughly. Cellulose oleates with degrees of substitution exceeding 1.23 exhibited amorphous structures and thermoplasticity with glass transition temperatures at 159.8 to 172.6 °C. This study presented a sustainable and practicable method for effectively derivatizing cellulose.

关键词： regenerated cellulose     cellulose oleate     sonochemistry     degree of substitution     thermoplasticity    

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Dynamic contribution of variable-speed wind energy conversion system in system frequency regulation

Yajvender Pal VERMA, Ashwani KUMAR

《能源前沿（英文）》 2012年 第6卷 第2期   页码 184-192 doi: 10.1007/s11708-012-0185-y

摘要： Frequency regulation in a generation mix having large wind power penetration is a critical issue, as wind units isolate from the grid during disturbances with advanced power electronics controllers and reduce equivalent system inertia. Thus, it is important that wind turbines also contribute to system frequency control. This paper examines the dynamic contribution of doubly fed induction generator (DFIG)-based wind turbine in system frequency regulation. The modified inertial support scheme is proposed which helps the DFIG to provide the short term transient active power support to the grid during transients and arrests the fall in frequency. The frequency deviation is considered by the controller to provide the inertial control. An additional reference power output is used which helps the DFIG to release kinetic energy stored in rotating masses of the turbine. The optimal speed control parameters have been used for the DFIG to increases its participation in frequency control. The simulations carried out in a two-area interconnected power system demonstrate the contribution of the DFIG in load frequency control.

关键词： doubly fed induction generator (DFIG)     load frequency control     inertial control     wind energy conversion system (WECS)    

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time on behavior of antibiotics and antibiotic resistance genes in aerobic granular reactor treating biogas

Jie Liao, Chaoxiang Liu, Lin Liu, Jie Li, Hongyong Fan, Jiaqi Ye, Zhichao Zeng

《环境科学与工程前沿（英文）》 2019年 第13卷 第3期 doi: 10.1007/s11783-019-1115-6

摘要：

Longer HRT can enhance degradation rate of sulfamethoxazole in granular reactor.

Longer HRT can reduce accumulated concentrations of TCs and QNs in sludge.

Longer HRT may have increased relative abundances of ARGs in aerobic granules.

关键词： Aerobic granules     Swine wastewater     Tetracyclines     Fluoroquinolones     Sulfonamides    

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Recent development in biogeotechnology and its engineering applications

《结构与土木工程前沿（英文）》 2021年 第15卷 第5期   页码 1073-1096 doi: 10.1007/s11709-021-0758-0

摘要： Microbial geotechnology or biogeotechnology is a new branch of geotechnical engineering. It involves the use of microbiology for traditional geotechnical applications. Many new innovative soil improvement methods have been developed in recent years based on this approach. A proper understanding of the various approaches and the performances of different methods can help researchers and engineers to develop the most appropriate geotechnical solutions. At present, most of the methods can be categorized into three major types, biocementation, bioclogging, and biogas desaturation. Similarities and differences of different approaches and their potential applications are reviewed. Factors affecting the different processes are also discussed. Examples of up-scaled model tests and pilot trials are presented to show the emerging applications. The challenges and problems of biogeotechnology are also discussed.

关键词： biogeotechnology     biocementation     bioclogging     biogas     strength enhancement     liquefaction mitigation     seepage control    

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Micro/nanofluidics-enabled energy conversion and its implemented devices

Yang YANG, Jing LIU

《能源前沿（英文）》 2011年 第5卷 第3期   页码 270-287 doi: 10.1007/s11708-010-0126-6

摘要： Most people were not aware of the role of energy as a basic force that drives the development and economic growth of the world until the two great oil crises occurred. According to the conservation law, energy not only exists in various forms but is also capable of being converted from one form to another. The common forms of energy are mechanical energy, chemical energy, internal energy, electrical energy, atomic energy, and electromagnetic energy, among others. The fluids in nature serve as the most common carriers and media in the energy conversion process. Following the rapid development of microelectromechanical systems (MEMS) technology, the energy supply and conversion issue in micro/nano scale has also been introduced in research laboratories worldwide. With unremitting efforts, great quantities of micro/nano scale energy devices have been investigated. Micro/nanofluid shows distinct features in transporting and converting energy similar to their counterpart macroscale tasks. In this paper, a series of micro/nanofluid-enabled energy conversion devices is reviewed based on the transformation between different forms of energy. The evaluation and contradistinction of their performances are also examined. The role of micro/nanofluid as media in micro/nano energy devices is summarized. This contributes to the establishment of a comprehensive and systematic structure in the relationship between energy conversion and fluid in the micro/nano scale. Some fundamental and practical issues are outlined, and the prospects in this challenging area are explored.

关键词： micro/nanofluid     different energy forms     energy conversion     medium role    

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标题 作者 时间 类型 操作

Techno-economic evaluation of a biogas-based oxidative coupling of methane process for ethylene production

Alberto T. Penteado, Mijin Kim, Hamid R. Godini, Erik Esche, Jens-Uwe Repke

期刊论文

Dehydration of natural gas and biogas streams using solid desiccants: a review

Soheil Bahraminia, Mansoor Anbia, Esmat Koohsaryan

期刊论文

Distribution of PCDD/Fs in a food waste anaerobic digestion process with biogas utilization

期刊论文

大型养殖场沼气工程

潘文智

期刊论文

Influence of HS and NH on biogas dry reforming using Ni catalyst: a study on single and synergetic effect

期刊论文

VALORIZATION OF BIOGAS THROUGH SIMULTANEOUS CO AND HS REMOVAL BY RENEWABLE AQUEOUS AMMONIA SOLUTION IN

期刊论文

Techno-economic assessment of providing control energy reserves with a biogas plant

Ervin Saracevic, David Woess, Franz Theuretzbacher, Anton Friedl, Angela Miltner

期刊论文

Biogas and its opportunities—A review

Panagiotis G. Kougias, Irini Angelidaki

期刊论文

Hydrogel photocatalysts for efficient energy conversion and environmental treatment

期刊论文

Biological conversion pathways of sulfate reduction ammonium oxidation in anammox consortia

Zhen Bi, Deqing Wanyan, Xiang Li, Yong Huang

期刊论文

Sustainable conversion regenerated cellulose into cellulose oleate by sonochemistry

期刊论文

Dynamic contribution of variable-speed wind energy conversion system in system frequency regulation

Yajvender Pal VERMA, Ashwani KUMAR

期刊论文

time on behavior of antibiotics and antibiotic resistance genes in aerobic granular reactor treating biogas

Jie Liao, Chaoxiang Liu, Lin Liu, Jie Li, Hongyong Fan, Jiaqi Ye, Zhichao Zeng

期刊论文

Recent development in biogeotechnology and its engineering applications

期刊论文

Micro/nanofluidics-enabled energy conversion and its implemented devices

Yang YANG, Jing LIU

期刊论文